New PDF release: A Bijective Proof of Kadell's Conjecture on Plane Partitions

By Kim D.

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Extra resources for A Bijective Proof of Kadell's Conjecture on Plane Partitions

Example text

This key elimination regenerated the mediator for the initial dehalogenation. This very fine tuning of the radical reactivities is the key element that makes the whole process work. Jang et al. reported a highly diastereoselective tandem radical reaction to prepare E-polysubstituted homoallylic alcohols (Scheme 64) [175]. This new process relies on the initial addition of benzoyl radicals onto an olefin. The intermediate radicals such as 201 underwent a stereoselective vinylation (two elementary steps) to form the desired Bz-protected homoallylic alcohols in good yields.

Similar strategies were used by Booker-Milburn et al. in approaches toward the synthesis of dictyol C and α-eudesmol [215], and by Blake et al. in approaches toward the synthesis of ophiobolin F and fusicoccin A [216]. , who showed that aryl-cyclopropylamines easily obtained by a Kulinkovich cyclopropanation could also undergo the oxidative fragmentation/cyclization reaction (Scheme 76) [217]. 0] framework treatment by a phosphite. Optimized conditions involve the use of silica gel in a fluorous solvent, which acts as an oxygen stock.

This key elimination regenerated the mediator for the initial dehalogenation. This very fine tuning of the radical reactivities is the key element that makes the whole process work. Jang et al. reported a highly diastereoselective tandem radical reaction to prepare E-polysubstituted homoallylic alcohols (Scheme 64) [175]. This new process relies on the initial addition of benzoyl radicals onto an olefin. The intermediate radicals such as 201 underwent a stereoselective vinylation (two elementary steps) to form the desired Bz-protected homoallylic alcohols in good yields.

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A Bijective Proof of Kadell's Conjecture on Plane Partitions by Kim D.


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